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https://www.mdpi.com/journal/polymers/special_issues/4CP14XFX3M Polymerized ionic liquids or poly(ionic liquids) (PILs) are a special type of polyelectrolytes that preserve the properties of ILs in each repeating structural unit. The main advantages of using PILs instead of ILs are their increased mechanical stability, durability and spatial controllability when compared to ILs. PILs produce films, membranes, coatings and fibers with the properties of ILs. The wide choice of pairs of cations and anions in PILs can be used to adjust the solubility of the polyelectrolyte, as well as its hydrophilicity, ionic conductivity, and heat resistance. The topics of this Special Issue are focused around the following: Electrolytes for electrochemical devices and PILs; Supercapacitors and polymer transistors; Catalysis and Chemical sensors and selective electrodes; Sorption and separation of gases and liquid-phase sorption This Special Issue is focused on a wide audience of researchers who want to learn more about the study and application of polymerized ionic liquids. Authors are welcome to submit their latest results in the form of original full articles, communications, or reviews on this wide topic.