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The report presents a study of aspects of using single and multiple output artificial neural networks to determine concentrations of inorganic salts in multi-component water solutions by processing their Raman spectra. The dependence of the results on complexity of the in- verse problem has been demonstrated. The results are compared for two data arrays including spectra of solutions of: 1) 5 salts composed of 10 different ions, and 2) 10 salts composed of 10 different ions.