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The enthalpies of formation of some azidocontaining compounds were determined. A new method for calculating the enthalpies of formation of aromatic radicals and the bond dissociation energies was proposed. The enthalpies of formation of azido- and azoradicals were determined. The energies of reorganization of these radicals were calculated. The sums of the energies of the chemical bonds in the molecular moieties transformed into radicals upon the decomposition of chemical compounds were found to be constant for different compounds.