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The ferroelectric and piezoelectric properties of ceramic solid solutions having a composition of (1−x)(Bi0.9Nd0.1)(Sc0.9 B 0.1)O3 − x PbTiO3 (x = 0.60–0.66; B = Lu, Yb, Er, Y) and obtained by solid state reaction were studied. An increase in the Curie temperature was found upon an increase in the concentration of lead titanate, while a drop occured upon the doping of the A and B sublattices. It was shown that at high temperatures, MnO2 and Bi2O3 additives lead to a reduction in the total conductivity and a dielectric loss of less than one order of magnitude. In modified ceramics, an increase in the d 33 and k t piezoelectric coefficients was observed as well. The effects of dielectric relaxation that are determined by the composition of the ceramics were revealed.