Application of Zeolite-Containing Catalysts for Plasma-Assisted Carbon Dioxide Reforming of Methaneстатья
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Дата последнего поиска статьи во внешних источниках: 20 февраля 2024 г.
Аннотация:The plasma-assisted process of dry reforming of methane in barrier discharge was studied using new compositions of zeolite-containing catalysts. Catalysts based on Ni, Fe, Co oxides promoted with CeO2 have been synthesize and characterized by low-temperature nitrogen adsorption–desorption, X-ray fluorescence spectroscopy, X-ray diffraction analysis, and temperature-programmed desorption of ammonia. The catalytic activity of the prepared samples on the reaction of the syngas production in gas discharge without additional heating of the reactor was studied. It was found that introduction of a catalyst into the discharge region makes it possible to increase the CH4 conversion from 10 to 16%, but has almost no effect on the CO2 conversion. In the presence of Fe-containing samples, the yield of CO and H2 decreases.